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Fabrication of shuttle-junctions for nanomechanical transfer of electrons

A V Moskalenko et al 2009 Nanotechnology 20 485202 (7pp)   doi: 10.1088/0957-4484/20/48/485202  Help

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A V Moskalenko1, S N Gordeev1, O F Koentjoro2, P R Raithby2, R W French2, F Marken2 and S Savel'ev3
1 Department of Physics, University of Bath, Claverton Down Road, Bath BA2 7AS, UK
2 Department of Chemistry, University of Bath, Claverton Down, Bath BA2 7AS, UK
3 Department of Physics, Loughborough University, Loughborough LE11 3TU, UK
E-mail: A.Moskalenko@bath.ac.uk

Abstract. We report on the fabrication of nanomechanical devices for shuttling of electrons from one electrode to another. Each device consists of a 20 nm diameter gold nanoparticle embedded within the gap between two gold electrodes. In two different kinds of shuttle-junctions the nanoparticle is attached to the electrodes through either (i) a single layer of 1,8-octanedithiol or (ii) a multilayer of 1-octanethiol molecules. The thiol layers play the role of 'damped springs', such that when a sufficient voltage bias is applied to the junction, the nanoparticle is expected to start oscillating and thereby transferring electrons from one electrode to the other. For both kinds of shuttle-junctions we observed an abrupt increase in the transmitted current above a threshold voltage, which can be attributed to a transition from the stationary to the oscillating regime. The threshold voltage was found to be lower for single-layer shuttle-junctions.

Print publication: Issue 48 (2 December 2009)
Received 20 August 2009
Published 4 November 2009

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