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Superparamagnetic relaxation in iron nanoclusters measured by low energy muon spin rotation

T J Jackson et al 2000 J. Phys.: Condens. Matter 12 1399-1411   doi: 10.1088/0953-8984/12/7/321  Help

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T J Jackson-+, C Binns++, E M Forgan-+, E Morenzoni§, Ch Niedermayer||, H Glückler§, A Hofer||§+, H Luetkens§¶, T Prokscha§, T M Riseman-+, A Schatz§¶, M Birke§¶, J Litterst¶, G Schatz|| and H P Weber§
-+ Condensed Matter Group, School of Physics and Astronomy, University of Birmingham, Birmingham B15 2TT, UK
++ Department of Physics and Astronomy, University of Leicester, Leicester LE1 7RH, UK
§ Paul Scherrer Institut, CH-5232 Villigen PSI, Switzerland
|| Fakultät für Physik, Universität Konstanz, D-78434 Konstanz, Germany
¶ Institut für Metallphysik und nukleare Festkörperphysik, Technische Universität Braunschweig, D-38106 Braunschweig, Germany
+ Tanner Documents, D-88131 Lindau, Germany
E-mail: t.j.jackson@bham.ac.uk

Abstract. Low energy (16 keV) muons were used to probe the dynamic magnetic behaviour of iron nanoclusters embedded in a silver thin film matrix. The silver film was 500 nm thick and contained a volume fraction of 0.1% iron. Measurements were made in a field of 25 mT, applied normal to the plane of the film, in the temperature range 4.7 K to 300 K. At temperatures above 20 K thermal activation of the cluster moments was seen as a narrowing of the field distribution sensed by the implanted muons. An intrinsic cluster relaxation time of τ0 = 12 ± 4 ns and an activation energy of 51 ± 9 K were deduced from fits to the data. SQUID magnetometry of thicker (1.5 µm) but otherwise identical films on graphite substrates showed the clusters to have a volume of the order of 10-26 m3, from which a cubic anisotropy constant of K = 2.3 ± 0.4 × 105 J m-3 was calculated. Remanence measurements showed no evidence of a preferred orientation for the magnetization of the cluster assembly.

Print publication: Issue 7 (21 February 2000)
Received 25 November 1999

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