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RAPID COMMUNICATION

Laser-driven photo-transmutation of 129I—a long-lived nuclear waste product

K W D Ledingham et al 2003 J. Phys. D: Appl. Phys. 36 L79-L82   doi: 10.1088/0022-3727/36/18/L01  Help

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K W D Ledingham1,6, J Magill2, P McKenna1, J Yang1, J Galy2, R Schenkel2, J Rebizant2, T McCanny1, S Shimizu1, L Robson1, R P Singhal3, M S Wei4, S P D Mangles4, P Nilson4, K Krushelnick4, R J Clarke5 and P A Norreys5
1 Department of Physics, University of Strathclyde, Glasgow G4 0NG, UK
2 European Commission, Joint Research Centre, Institute for Transuranium Elements, Postfach 2340, 76125 Karlsruhe, Germany
3 Department of Physics and Astronomy, University of Glasgow, Glasgow G12 8QQ, UK
4 Blackett Laboratory, Imperial College, London SW7 2BZ, UK
5 Central Laser Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxon OX11 0QX, UK
6 Also at AWE plc Aldermaston, Reading RG7 4PR, UK.
E-mail: k.ledingham@phys.strath.ac.uk

Abstract. Intense laser–plasma interactions produce high brightness beams of gamma rays, neutrons and ions and have the potential to deliver accelerating gradients more than 1000 times higher than conventional accelerator technology, and on a tabletop scale. This paper demonstrates one of the exciting applications of this technology, namely for transmutation studies of long-lived radioactive waste. We report the laser-driven photo-transmutation of long-lived 129I with a half-life of 15.7 million years to 128I with a half-life of 25 min. In addition, an integrated cross-section of 97 ± 40 mbarns for the reaction 129I(γ, n)128I is determined from the measured ratio of the (γ, n) induced 128I and 126I activities. The potential for affordable, easy to shield, tabletop laser technology for nuclear transmutation studies is highlighted.

Print publication: Issue 18 (21 September 2003)
Received 12 August 2003
Published 3 September 2003

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