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Multiphoton dynamics and resonance lineshapes in three-level systems: many-mode Floquet treatment

Kwanghsi Wang et al 1985 J. Phys. B: At. Mol. Phys. 18 4539-4556   doi: 10.1088/0022-3700/18/23/008  Help

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Kwanghsi Wang, Tak-San Ho and Shih-I Chu
Dept. of Chem., Kansas Univ., Lawrence, KS, USA

Abstract. The authors present an exact treatment of two- and multiquantum transitions in three-level systems driven by two intense linearly polarised monochromatic fields based on the semiclassical many-mode Floquet theory developed recently. Further they extend the almost degenerate perturbation theory of Salwen (1955-6) to the two-mode Floquet Hamiltonian and obtain approximate analytical formulae for multiphoton transition probabilities, resonance bichromatic shifts and widths, and absorption lineshapes beyond the conventional rotating-wave approximation (RWA). Detailed comparison of the analytical, the RWA, and the exact results is given. Several novel features of multiphoton lineshape characteristics are pointed out.

Print publication: Issue 23 (14 December 1985)

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